Homogeneous solution assembled Turing structures with near zero strain semi-coherence interface

Constructing a Turing structure in homogeneous solutions is a large challenge because of the similar diffusion coefficients of most small molecule weight species. Here, we show that Turing structure with near zero strain semi-coherence interfaces is constructed subject to the diffusion kinetics.

Published in Physics

Homogeneous solution assembled Turing structures with near zero strain semi-coherence interface
Like

Share this post

Choose a social network to share with, or copy the URL to share elsewhere

This is a representation of how your post may appear on social media. The actual post will vary between social networks

Numerous natural systems contain surfaces or threads that enable directional interface contact, such as zebra stripes, spot fish, and undulating sand dunes. Some spatiotemporal stationary structures, which are summarized by Alan Turing as the interaction of reaction and diffusion with each othe. Turing explained the emergence of stationary patterns by invoking the interplay between an activator and an inhibitor with different diffusion rates, which has proven to be extremely influential across many disciplines because they can show enhanced features resulting from abundant and smooth interfaces. Recently, Tan used a facile route based on aqueous-organic interfacial polymerization to generate Turing-type polyamide membranes for water purification, and these membranes exhibit excellent water-salt separation performance. Zhang reported a cation exchange approach in the heterogeneous solvent of diethylenetriamine and deionized water to produce Turing-type Ag2Se on CoSe2 nanobelts relied on diffusion-driven instability, which is highly effective in catalyzing the oxygen evolution reaction (OER) in alkaline electrolytes with an 84.5% anodic energy efficiency. It should be noted that the above case studies the related potential of the Turing structure in heterogeneous solution. However, to date, realization of an inorganic Turing structure (spots or stripes) in homogeneous solutions has not been reported because of the similar diffusion coefficients for most small molecule weight species.

Fig. 1 a, SEM image of spots Turing Structure (Zn:Fe=1:3).  b, SEM image of stripes Turing Structure (Zn:Fe=1:6).c, Three-dimensional APT volume (20× 20 × 80 nm3) of the center of the Turing interface film (Zn: Fe=1:3). d, Combined and individual atom distribution maps. e, One-dimensional concentration profile taken along the arrow in c.

Fig. 1a and b show the spot-like and stripe-like Turing structures prepared with Zn-Fe-O as a model, and Fig. 1c–e can clearly observe the existence of the ZnFe2O4/α-Fe2O3 dual-phase interface. Fig. 2 shows the evolution of the Turing structure at different diffusion coefficient differences or different starting positions, which are well matched with the experimental microstructure, so it can be confirmed that this phase separation is a Turing structure and is influenced by reaction diffusion theory modulation. Therefore, more mathematical models or parameters can be introduced to obtain more Turing structured films, bringing new approaches for chemical and material design.

Fig. 2 Patterns exhibited by the numerical  simulated by the predator model at different discrete time (T=1, 100, 600, and 1000). a, Diffusion coefficients differ by a factor of 30. b, Diffusion coefficients differ by a factor of 30, and the initial position is changed. c, Diffusion coefficients differ by a factor of 20.

Please sign in or register for FREE

If you are a registered user on Research Communities by Springer Nature, please sign in

Follow the Topic

Physics and Astronomy
Physical Sciences > Physics and Astronomy

Related Collections

With Collections, you can get published faster and increase your visibility.

Clinical trials 2025

In this cross-journal Collection between Nature Communications, Communications Medicine, and Scientific Reports we invite submission of clinical trials.

Publishing Model: Open Access

Deadline: Dec 31, 2025

Women's Health

A selection of recent articles that highlight issues relevant to the treatment of neurological and psychiatric disorders in women.

Publishing Model: Hybrid

Deadline: Ongoing